Scattering and imaging with x-ray beams carrying orbital angular momentum

Apr 17, 2024, 3:30 PM
30m
Oral

Speaker

Maurizio Sacchi (CNRS-INSP and Synchrotron SOLEIL)

Description

The interaction of light beams with magnetic materials defines the rich set of analytical tools in magneto-optics, covering photon energies from infra-red to hard x-rays. In addition to the spin angular momentum (SAM) associated to the light polarization, Laguerre-Gaussian (LG) beams carry also an orbital angular momentum (OAM) of ℓℏ/photon [1] associated to an azimuthal dependence exp(iℓϕ) of the electric field phase. Over the last thirty years, OAM beams at vis-IR wavelengths found applications in biology, telecommunication, imaging and quantum technologies [2]. Their capability to exert a mechanical torque was exploited to create optical spanners for manipulating small particles. The azimuthal phase dependence introduces a singularity on the propagation axis and a radial modulation of the intensity (ring-shaped), properties that have been used to modify magnetic ordering, to improve the spatial resolution in microscopy, and to enhance the edge sharpness in phase-contrast imaging. Over the last decade, the generation of OAM beams at shorter wavelengths, from XUV to hard x-rays, is also finding an increasing number of applications, often based on extrapolations of previous work carried out in the visible range. For instance, as it happened for the SAM, the handedness imposed by the OAM has been exploited to perform x-ray spectroscopic studies of magnetic materials [3] and of chiral molecules [4], and a recent ptychography study [5] showed that the attainable spatial resolution in the reconstructed XUV images increases with ℓ. All these extensions of the use of OAM beams from the visible to the x-rays open new perspectives for element selective spectroscopy and imaging of magnetic structures.

[1].L. Allen at al., Orbital angular momentum of light and the transformation of Laguerre-Gaussian laser modes, Phys. Rev. A 45, 8185 (1992). [2]. Y. Shen et al., Optical vortices 30 years on: OAM manipulation from topological charge to multiple singularities, Light: Science & Applications 8, 90 (2019) [3]. M. Fanciulli et al., Electromagnetic theory of Helicoidal Dichroism in reflection from magnetic structures, Phys. Rev. A 103, 013501 (2021); T. Ruchon, M. Fanciulli, M. Sacchi, Magneto-Optics with light beams carrying orbital angular momentum, in The 2022 magneto-optics roadmap , J. Phys. D: Appl. Phys. 55, 463003 (2022); M. Fanciulli et al., Observation of magnetic helicoidal dichroism with extreme ultraviolet light vortices, Phys. Rev. Lett. 128, 077401 (2022). [4]. J. R. Rouxel et al., Hard X-ray helical dichroism of disordered molecular media, Nature Photonics 16, 570 (2022).[5]. M. Pancaldi et al., High-resolution ptychographic imaging at a seeded free-electron laser source using OAM beams, Optica 11, 403 (2024).

M.Pancaldi(1,2), M.Fanciulli(3,4), A.E.Stanciu(5), M.Guer(4), C.Spezzani(1), E.Pedersoli(1), M.Luttmann(4), M.Vimal(4), D.Bresteau(4), D.DeAngelis(1), P.R.Ribic(1), B.Rösner(7), C.David(7), M.Manfredda(1), F.Guzzi(1), C.B.Bevis(8), J.Barolak(9), S.Bonetti(2), I.Bykova(7), L.Novinec(1), A.Ravindran(10), A.Simoncig(1), D.E.Adams(9), G.Kourousias(1), G.Mancini(8), P.Vavassori(11), R.Sousa(5), I-L.Prejbeanu(5), L.Vila(5), L.Buda-Prejbeanu(5), B.Dieny(5), G.DeNinno(1,10), F.Capotondi(1), T.Ruchon(4), M.Sacchi(6,12)

1 ELETTRA – Sincrotrone Trieste ... 2 Università di Ca’ Foscari, Venezia ..... 3 LPMS – Cergy Paris Université
4 Lidyl – AttoLab, CEA Saclay .... 5 Spintec, CEA Grenoble ... 6 CNRS – INSP, Sorbonne Université Paris
7 Paul Scherrer Institut, Villigen ...... 8 LUXEM, Università di Pavia .... 9 Colorado School of Mines, Golden
10 LQO, University of Nova Gorica ..... 11 CIC-NanoGune San Sebastian and IKERBASQUE Bilbao
12 Synchrotron SOLEIL, Paris-Saclay

Primary author

Maurizio Sacchi (CNRS-INSP and Synchrotron SOLEIL)

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